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Biomimetic Based Applications by Anne George

By Anne George

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Y. ; Valentine, J. S. Inorg. Chem. 1996, 35, 10451049. [77] Zhou, X. ; Ji, H. B. Chem. Eng. J. 2010, 156, 411-417. ; Ishii, Y. Tetrahedron Lett. 1992, 33, 6827-6830. [79] Harvey, J. ; Ziegler, C. ; Krzystek, J. Inorg. Chem. 2005, 44, 4451-4453. [80] Goldberg, D. ; Montalban, A. ; Brunel, L. ; Barrett, A. G. ; Hoffman, B. M. J. Am. Chem. Soc. 1997, 119, 8722-8723. [81] Lansky, D. ; Zvyagin, S. ; Kadish, K. ; Rheingold, A. ; Goldberg, D. P. Inorg. Chem. 2005, 44, 4485-4498. [82] Caudle, M. ; Mobley, C.

3 Cyclohexene Conv. 7×104 Table 5. 3×10-5mol/L cobalt tetraphenylporphyrin. 2 Biomimetic oxidation of C=C of styrene In 2006, We[75] reported a novel aerobic oxidative cleavage of C=C double bonds of styrene catalyzed by simple manganese porphyrin(Scheme 6). H manganese porphyrin O O + + other products T,P Scheme 6. Aerobic oxidation of styrene by metalloporphyrin Under the catalysis of chloro(tetraphenylporphinato)manganese, the oxidative cleavage of the carbon-carbon double bond of the styrene with air yields the main product benzaldehyde.

We tried to use the simple μ-oxobismetalloporphyrin (TPPFeIII)2O to catalyze hydroxylation of hydrocarbons using air as the terminal oxidant to gain a better understanding of the possibility of using simple μ-oxo dimeric metalloporphyrin to catalyze the hydrocarbon oxidation directly by air. We developed a new reaction system for the aerobic oxidation of the inactive C-H bond of cyclohexane catalyzed by a very small amount of simple μ-oxo-ironporphyrin (TPPFeIII)2O[53](Scheme 1). OH (TPPFeIII) + O2 2O O + + H 2O T/P Scheme 1.

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